Subpicosecond conformational dynamics of small peptides probed by two-dimensional vibrational spectroscopy.

Woutersen, S; Mu, Y; Stock, G; Hamm, P · Proc Natl Acad Sci U S A · 2001

basic_science · Level V

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Abstract

The observation of subpicosecond fluctuations in the conformation of a small peptide in water is demonstrated. We use an experimental method that is specifically sensitive to conformational dynamics taking place on an ultrafast time scale. Complementary molecular-dynamics simulations confirm that the conformational fluctuations exhibit a subpicosecond component, the time scale and amplitude of which agree well with those derived from the experiment.

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