Polarization-dependent optical 2D Fourier transform spectroscopy of semiconductors.

Zhang, Tianhao; Kuznetsova, Irina; Meier, Torsten; Li, Xiaoqin; Mirin, Richard P; Thomas, Peter; Cundiff, Steven T · Proc Natl Acad Sci U S A · 2007

basic_science · Level V

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Abstract

Optical 2D Fourier transform spectroscopy (2DFTS) provides insight into the many-body interactions in direct gap semiconductors by separating the contributions to the coherent nonlinear optical response. We demonstrate these features of optical 2DFTS by studying the heavy-hole and light-hole excitonic resonances in a gallium arsenide quantum well at low temperature. Varying the polarization of the incident beams exploits selection rules to achieve further separation. Calculations using a full many-body theory agree well with experimental results and unambiguously demonstrate the dominance of many-body physics.

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