Structure of the buried metal-molecule interface in organic thin film devices.

Hansen, Christian R; Sørensen, Thomas J; Glyvradal, Magni; Larsen, Jacob; Eisenhardt, Sara H; Bjørnholm, Thomas; Nielsen, Martin M; Feidenhans'l, Robert et al. · Nano Lett · 2009

basic_science · Level V

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Abstract

By use of specular X-ray reflectivity (XR) the structure of a metal-covered organic thin film device is measured with angstrom resolution. The model system is a Langmuir-Blodgett (LB) film, sandwiched between a silicon substrate and a top electrode consisting of 25 A titanium and 100 A aluminum. By comparison of XR data for the five-layer Pb2+ arachidate LB film before and after vapor deposition of the Ti/Al top electrode, a detailed account of the structural damage to the organic film at the buried metal-molecule interface is obtained. We find that the organized structure of the two topmost LB layers (approximately 5 nm) is completely destroyed due to the metal deposition.

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