Nanoporous pt-co alloy nanowires: fabrication, characterization, and electrocatalytic properties.

Liu, Lifeng; Pippel, Eckhard; Scholz, Roland; Gösele, Ulrich · Nano Lett · 2009

basic_science · Level V

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Abstract

Nanoporous Pt-Co alloy nanowires were synthesized by electrodeposition of Co-rich Pt(1)Co(99) alloy into anodic aluminum oxide (AAO) membranes, followed by a dealloying treatment in a mild acidic medium. These nanowires consist of porous skeletons with tiny pores of 1-5 nm and crystalline ligaments of 2-8 nm. Morphological and compositional evolutions of the porous Pt-Co nanowires upon dealloying were investigated, and their formation mechanism is discussed. The nanoporous Pt-Co alloy nanowires are found to exhibit distinctly enhanced electrocatalytic activities toward methanol oxidation as compared to the current state-of-the-art Pt/C and PtCo/C catalysts, thus showing substantial promise as efficient anode electrocatalysts in direct methanol fuel cells.

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