Calcium-decorated graphene-based nanostructures for hydrogen storage.

Lee, Hoonkyung; Ihm, Jisoon; Cohen, Marvin L; Louie, Steven G · Nano Lett · 2010

basic_science · Level V

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Abstract

We report a first-principles study of hydrogen storage media consisting of calcium atoms and graphene-based nanostructures. We find that Ca atoms prefer to be individually adsorbed on the zigzag edge of graphene with a Ca-Ca distance of 10 A without clustering of the Ca atoms, and up to six H(2) molecules can bind to a Ca atom with a binding energy of approximately 0.2 eV/H(2). A Ca-decorated zigzag graphene nanoribbon (ZGNR) can reach the gravimetric capacity of approximately 5 wt % hydrogen. We also consider various edge geometries of the graphene for Ca dispersion.

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