Observation of breathing-like modes in an individual multiwalled carbon nanotube.

Spudat, Christian; Müller, Matthias; Houben, Lothar; Maultzsch, Janina; Goss, Karin; Thomsen, Christian; Schneider, Claus M; Meyer, Carola · Nano Lett · 2010

basic_science · Level V

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Abstract

We study collective vibrational breathing modes in the Raman spectrum of a multiwalled carbon nanotube. In correlation with high-resolution transmission electron microscopy, we find that these modes have energies differing by more than 23% from the radial breathing modes of the corresponding single-walled nanotubes. This shift in energy is explained with intershell interactions using a model of coupled harmonic oscillators. The strength of this interaction is related to the coupling strength expected for few-layer graphene.

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