Self-assembly of metal nanostructures on binary alloy surfaces.

Duguet, T; Han, Yong; Yuen, Chad; Jing, Dapeng; Unal, Barış; Evans, J W; Thiel, P A · Proc Natl Acad Sci U S A · 2011

basic_science · Level V

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Abstract

Deposition of metals on binary alloy surfaces offers new possibilities for guiding the formation of functional metal nanostructures. This idea is explored with scanning tunneling microscopy studies and atomistic-level analysis and modeling of nonequilibrium island formation. For Au/NiAl(110), complex monolayer structures are found and compared with the simple fcc(110) bilayer structure recently observed for Ag/NiAl(110). We also consider a more complex codeposition system, (Ni + Al)/NiAl(110), which offers the opportunity for fundamental studies of self-growth of alloys including deviations for equilibrium ordering. A general multisite lattice-gas model framework enables analysis of structure selection and morphological evolution in these systems.

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