Discrete dynamics of nanoparticle channelling in suspended graphene.

Booth, Tim J; Pizzocchero, Filippo; Andersen, Henrik; Hansen, Thomas W; Wagner, Jakob B; Jinschek, Joerg R; Dunin-Borkowski, Rafal E; Hansen, Ole et al. · Nano Lett · 2011

basic_science · Level V

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Abstract

We have observed a previously undescribed stepwise oxidation of mono- and few layer suspended graphene by silver nanoparticles in situ at subnanometer scale in an environmental transmission electron microscope. Over the range of 600-850 K, we observe crystallographically oriented channelling with rates in the range 0.01-1 nm/s and calculate an activation energy of 0.557 ± 0.016 eV. We present a discrete statistical model for this process and discuss the implications for accurate nanoscale patterning of nanoscale systems.

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