Valence state-dependent ferromagnetism in Mn-doped NiO thin films.

Yan, Wensheng; Sun, Zhihu; Li, Zhongrui; Liu, Qinghua; Yao, Tao; Pan, Zhiyun; Wang, Chao; Hu, Fengchun et al. · Adv Mater · 2012

basic_science · Level V

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Abstract

Manipulating the ferromagnetism of diluted magnetic semiconductors by tuning the valence state of doped ions is found to be achievable in Mn-doped NiO. First-principles calculations predict that the interactions between substitutional Mn(3+) ions in NiO are ferromagnetic, while the Mn(2+)-Mn(2+) interactions are antiferromagnetic. This scenario is experimentally supported by a great enhancement of saturation magnetization with increased Mn(3+)/Mn(2+) ratio in Mn-doped and (Mn, Li)-codoped NiO.

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