Exciton-plasmon interactions in quantum dot-gold nanoparticle structures.

Cohen-Hoshen, Eyal; Bryant, Garnett W; Pinkas, Iddo; Sperling, Joseph; Bar-Joseph, Israel · Nano Lett · 2012

basic_science · Level V

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Abstract

We present a self-assembly method to construct CdSe/ZnS quantum dot-gold nanoparticle complexes. This method allows us to form complexes with relatively good control of the composition and structure that can be used for detailed study of the exciton-plasmon interactions. We determine the contribution of the polarization-dependent near-field enhancement, which may enhance the absorption by nearly two orders of magnitude and that of the exciton coupling to plasmon modes, which modifies the exciton decay rate.