Selective molecular transport through intrinsic defects in a single layer of CVD graphene.

O'Hern, Sean C; Stewart, Cameron A; Boutilier, Michael S H; Idrobo, Juan-Carlos; Bhaviripudi, Sreekar; Das, Sarit K; Kong, Jing; Laoui, Tahar et al. · ACS Nano · 2012

basic_science · Level V

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Abstract

We report graphene composite membranes with nominal areas more than 25 mm(2) fabricated by transfer of a single layer of CVD graphene onto a porous polycarbonate substrate. A combination of pressure-driven and diffusive transport measurements provides evidence of size-selective transport of molecules through the membrane, which is attributed to the low-frequency occurrence of intrinsic 1-15 nm diameter pores in the CVD graphene. Our results present the first step toward the realization of practical membranes that use graphene as the selective material.

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