Amplified spontaneous emission in conjugated polyrotaxanes under quasi-CW pumping.

Mróz, Marta M; Sforazzini, Giuseppe; Zhong, Yongchun; Wong, Kam Sing; Anderson, Harry L; Lanzani, Guglielmo; Cabanillas-Gonzalez, Juan · Adv Mater · 2013

basic_science · Level V

Where this comes from

Abstract

Amplified spontaneous emission under millisecond pulsed excitation on a rotaxane-insulated conjugated polymer is reported. Pump-probe spectroscopy confirms the absence of polaron-pair absorption in the gain spectral region as the main factor contributing to quasi-steady-state amplified spontaneous emission. The low polaron-pair yield in this compound is the likely result of effective backbone encapsulation provided by the threading ring.