Hollow structured Li3VO4 wrapped with graphene nanosheets in situ prepared by a one-pot template-free method as an anode for lithium-ion batteries.

Shi, Yi; Wang, Jia-Zhao; Chou, Shu-Lei; Wexler, David; Li, Hui-Jun; Ozawa, Kiyoshi; Liu, Hua-Kun; Wu, Yu-Ping · Nano Lett · 2013

basic_science · Level V

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Abstract

To explore good anode materials of high safety, high reversible capacity, good cycling, and excellent rate capability, a Li3VO4 microbox with wall thickness of 40 nm was prepared by a one-pot and template-free in situ hydrothermal method. In addition, its composite with graphene nanosheets of about six layers of graphene was achieved. Both of them, especially the Li3VO4/graphene nanosheets composite, show superior electrochemical performance to the formerly reported vanadium-based anode materials. The composite shows a reversible capacity of 223 mAh g(-1) even at 20C (1C = 400 mAh g(-1)). After 500 cycles at 10C there is no evident capacity fading.