Plasmonic surface lattice resonances at the strong coupling regime.
basic_science · Level V
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- Record sourced from PubMed, PMID 24279840.
- Also identified by DOI 10.1021/nl4035219.
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Abstract
We show strong coupling involving three different types of resonances in plasmonic nanoarrays: surface lattice resonances (SLRs), localized surface plasmon resonances on single nanoparticles, and excitations of organic dye molecules. The measured transmission spectra show splittings that depend on the molecule concentration. The results are analyzed using finite-difference time-domain simulations, a coupled-dipole approximation, coupled-modes models, and Fano theory. The delocalized nature of the collective SLR modes suggests that in the strong coupling regime molecules near distant nanoparticles are coherently coupled.