Nanostructured singlet fission photovoltaics subject to triplet-charge annihilation.

Thompson, Nicholas J; Hontz, Eric; Congreve, Daniel N; Bahlke, Matthias E; Reineke, Sebastian; Van Voorhis, Troy; Baldo, Marc A · Adv Mater · 2014

basic_science · Level V

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Abstract

Singlet exciton fission is an efficient multiple-exciton generation process that is vulnerable to a characteristic loss process: triplet-charge annihilation. This loss process is characterized in singlet-fission photovoltaics and losses as high as 40% are observed in poorly designed devices. Techniques are demonstrated to improve charge extraction and reduce triplet-charge annihilation to negligible levels at short-circuit conditions.