Directed assembly of lamellae forming block copolymer thin films near the order-disorder transition.

Kim, Sangwon; Nealey, Paul F; Bates, Frank S · Nano Lett · 2014

basic_science · Level V

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Abstract

The impact of thin film confinement on the ordering of lamellae was investigated using symmetric poly(styrene-b-[isoprene-ran-epoxyisoprene]) diblock copolymers bound by nonpreferential wetting interfaces. The order-disorder transition temperature (TODT) and the occurrence of composition fluctuations in the disordered state are not significantly affected by two-dimensional confinement. Directed self-assembly using chemical patterning is demonstrated near TODT. These results establish the minimum feature size attainable using directed self-assembly of a given diblock copolymer system.