Trap-induced losses in hybrid photovoltaics.

Gao, Feng; Li, Zhe; Wang, Jianpu; Rao, Akshay; Howard, Ian A; Abrusci, Agnese; Massip, Sylvain; McNeill, Christopher R et al. · ACS Nano · 2014

basic_science · Level V

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Abstract

We investigate the loss mechanisms in hybrid photovoltaics based on blends of poly(3-hexylthiophene) with CdSe nanocrystals of various sizes. By combining the spectroscopic and electrical measurements on working devices as well as films, we identify that high trap-mediated recombination is responsible for the loss of photogenerated charge carriers in devices with small nanocrystals. In addition, we demonstrate that the reduced open-circuit voltage for devices with small nanocrystals is also caused by the traps.