High charge carrier mobilities and lifetimes in organolead trihalide perovskites.

Wehrenfennig, Christian; Eperon, Giles E; Johnston, Michael B; Snaith, Henry J; Herz, Laura M · Adv Mater · 2014

basic_science · Level V

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Abstract

Organolead trihalide perovskites are shown to exhibit the best of both worlds: charge-carrier mobilities around 10 cm2 V−1 s−1 and low bi-molecular charge-recombination constants. The ratio of the two is found to defy the Langevin limit of kinetic charge capture by over four orders of magnitude. This mechanism causes long (micrometer) charge-pair diffusion lengths crucial for flat-heterojunction photovoltaics.