Ultrafast polarization response of an optically trapped single ferroelectric nanowire.

Nah, Sanghee; Kuo, Yi-Hong; Chen, Frank; Park, Joonsuk; Sinclair, Robert; Lindenberg, Aaron M · Nano Lett · 2014

basic_science · Level V

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Abstract

One-dimensional potassium niobate nanowires are of interest as building blocks in integrated piezoelectric devices, exhibiting large nonlinear optical and piezoelectric responses. Here we present femtosecond measurements of light-induced polarization dynamics within an optically trapped ferroelectric nanowire, using the second-order nonlinear susceptibility as a real-time structural probe. Large amplitude, reversible modulations of the nonlinear susceptibility are observed within single nanowires at megahertz repetition rates, developing on few-picosecond time-scales, associated with anomalous coupling of light into the nanowire.