Femtosecond all-optical synchronization of an X-ray free-electron laser.

Schulz, S; Grguraš, I; Behrens, C; Bromberger, H; Costello, J T; Czwalinna, M K; Felber, M; Hoffmann, M C et al. · Nat Commun · 2015

basic_science · Level V

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Abstract

Many advanced applications of X-ray free-electron lasers require pulse durations and time resolutions of only a few femtoseconds. To generate these pulses and to apply them in time-resolved experiments, synchronization techniques that can simultaneously lock all independent components, including all accelerator modules and all external optical lasers, to better than the delivered free-electron laser pulse duration, are needed. Here we achieve all-optical synchronization at the soft X-ray free-electron laser FLASH and demonstrate facility-wide timing to better than 30 fs r.m.s. for 90 fs X-ray photon pulses. Crucially, our analysis indicates that the performance of this optical synchronization is limited primarily by the free-electron laser pulse duration, and should naturally scale to the sub-10 femtosecond level with shorter X-ray pulses.