Large-Area Nanoimprinted Colloidal Au Nanocrystal-Based Nanoantennas for Ultrathin Polarizing Plasmonic Metasurfaces.

Chen, Wenxiang; Tymchenko, Mykhailo; Gopalan, Prashanth; Ye, Xingchen; Wu, Yaoting; Zhang, Mingliang; Murray, Christopher B; Alu, Andrea et al. · Nano Lett · 2015

basic_science · Level V

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Abstract

We report a low-cost, large-area fabrication process using solution-based nanoimprinting and compact ligand exchange of colloidal Au nanocrystals to define anisotropic, subwavelength, plasmonic nanoinclusions for optical metasurfaces. Rod-shaped, Au nanocrystal-based nanoantennas possess strong, localized, plasmonic resonances able to control polarization. We fabricate metasurfaces from rod-shaped nanoantennas tailored in size and spacing to demonstrate Au nanocrystal-based quarter-wave plates that operate with extreme bandwidths and provide high polarization conversion efficiencies in the near-to-mid infrared.

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