Observation of intervalley quantum interference in epitaxial monolayer tungsten diselenide.

Liu, Hongjun; Chen, Jinglei; Yu, Hongyi; Yang, Fang; Jiao, Lu; Liu, Gui-Bin; Ho, Wingking; Gao, Chunlei et al. · Nat Commun · 2015

basic_science · Level V

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Abstract

The extraordinary electronic structures of monolayer transition metal dichalcogenides, such as the spin-valley-coupled band edges, have sparked great interest for potential spintronic and valleytronic applications based on these two-dimensional materials. In this work, we report the experimental observation of quasi-particle interference patterns in monolayer WSe2 using low-temperature scanning tunnelling spectroscopy. We observe intervalley quantum interference involving the Q valleys in the conduction band due to spin-conserving scattering processes, while spin-flipping intervalley scattering is absent. Our results establish unequivocally the presence of spin-valley coupling and affirm the large spin splitting at the Q valleys. Importantly, the inefficient spin-flipping scattering implies long valley and spin lifetime in monolayer WSe2, which is a key figure of merit for valley-spintronic applications.