Ferromagnetism: Sulfur Doping Induces Strong Ferromagnetic Ordering in Graphene: Effect of Concentration and Substitution Mechanism (Adv. Mater. 25/2016).

Tuček, Jiří; Błoński, Piotr; Sofer, Zdeněk; Šimek, Petr; Petr, Martin; Pumera, Martin; Otyepka, Michal; Zbořil, Radek · Adv Mater · 2016

basic_science · Level V

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Abstract

R. Zbořil and co-workers show that doping a graphene lattice with sulfur induces magnetic centers which display ferromagnetic order below ≈62 K. As described on page 5045, sulfur doping promotes magnetically active configurations resembling the gamma-thiothiapyrone motif. Enhanced magnetic properties of sulfur-doped graphene are attributed to two unpaired electrons from each sulfur atom injected into the graphene conducting band where they are delocalized between the S and C atoms.