Two Dimensional Antiferromagnetic Chern Insulator: NiRuCl<sub>6</sub>.

Zhou, P; Sun, C Q; Sun, L Z · Nano Lett · 2016

basic_science · Level V

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Abstract

Density functional theory (DFT) and Berry curvature calculations show that quantum anomalous Hall effect (QAHE) can be realized in two-dimensional(2D) antiferromagnetic (AFM) NiRuCl<sub>6</sub>. The results indicate that NiRuCl<sub>6</sub> behaves as an AFM Chern insulator and its spin-polarized electronic structure and strong spin-orbit coupling (SOC) are responsible for the QAHE. By tuning SOC, we found that the topological property of NiRuCl<sub>6</sub> arises from its energy band inversion. Considering the compatibility between the AFM and insulators, AFM Chern insulator provides a new way to archive high temperature QAHE in experiments due to its different magnetic coupling mechanism from that of ferromagnetic (FM) Chern insulator.