Interface Engineering in Solution-Processed Nanocrystal Thin Films for Improved Thermoelectric Performance.

Ding, Defang; Wang, Dawei; Zhao, Man; Lv, Jiawei; Jiang, Hong; Lu, Chenguang; Tang, Zhiyong · Adv Mater · 2017

basic_science · Level V

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Abstract

Solution-processed PbTe nanocrystal (NC) thin films are ligand exchanged by ethylenediamine and then annealed at 400 °C for enhancement of NC coupling. To further improve the performance, heterostructures are introduced into the PbTe/PbS films. Significantly, an optimized ZT of ≈0.30 is successfully achieved at 405 K. This method opens an avenue toward thermoelectric thin film devices with high performance.