Large positive in-plane magnetoresistance induced by localized states at nanodomain boundaries in graphene.

Wu, Han-Chun; Chaika, Alexander N; Hsu, Ming-Chien; Huang, Tsung-Wei; Abid, Mourad; Abid, Mohamed; Aristov, Victor Yu; Molodtsova, Olga V et al. · Nat Commun · 2017

basic_science · Level V

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Abstract

Graphene supports long spin lifetimes and long diffusion lengths at room temperature, making it highly promising for spintronics. However, making graphene magnetic remains a principal challenge despite the many proposed solutions. Among these, graphene with zig-zag edges and ripples are the most promising candidates, as zig-zag edges are predicted to host spin-polarized electronic states, and spin-orbit coupling can be induced by ripples. Here we investigate the magnetoresistance of graphene grown on technologically relevant SiC/Si(001) wafers, where inherent nanodomain boundaries sandwich zig-zag structures between adjacent ripples of large curvature. Localized states at the nanodomain boundaries result in an unprecedented positive in-plane magnetoresistance with a strong temperature dependence. Our work may offer a tantalizing way to add the spin degree of freedom to graphene.