Giant tunnelling electroresistance in metal/ferroelectric/semiconductor tunnel junctions by engineering the Schottky barrier.

Xi, Zhongnan; Ruan, Jieji; Li, Chen; Zheng, Chunyan; Wen, Zheng; Dai, Jiyan; Li, Aidong; Wu, Di · Nat Commun · 2017

basic_science · Level V

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Abstract

Recently, ferroelectric tunnel junctions have attracted much attention due to their potential applications in non-destructive readout non-volatile memories. Using a semiconductor electrode has been proven effective to enhance the tunnelling electroresistance in ferroelectric tunnel junctions. Here we report a systematic investigation on electroresistance of Pt/BaTiO<sub>3</sub>/Nb:SrTiO<sub>3</sub> metal/ferroelectric/semiconductor tunnel junctions by engineering the Schottky barrier on Nb:SrTiO<sub>3</sub> surface via varying BaTiO<sub>3</sub> thickness and Nb doping concentration. The optimum ON/OFF ratio as great as 6.0 × 10<sup>6</sup>, comparable to that of commercial Flash memories, is achieved in a device with 0.1 wt% Nb concentration and a 4-unit-cell-thick BaTiO<sub>3</sub> barrier. With this thinnest BaTiO<sub>3</sub> barrier, which shows a negligible resistance to the tunnelling current but is still ferroelectric, the device is reduced to a polarization-modulated metal/semiconductor Schottky junction that exhibits a more efficient control on the tunnelling resistance to produce the giant electroresistance observed. These results may facilitate the design of high performance non-volatile resistive memories.