Coherent control of the silicon-vacancy spin in diamond.

Pingault, Benjamin; Jarausch, David-Dominik; Hepp, Christian; Klintberg, Lina; Becker, Jonas N; Markham, Matthew; Becher, Christoph; Atatüre, Mete · Nat Commun · 2017

basic_science · Level V

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Abstract

Spin impurities in diamond have emerged as a promising building block in a wide range of solid-state-based quantum technologies. The negatively charged silicon-vacancy centre combines the advantages of its high-quality photonic properties with a ground-state electronic spin, which can be read out optically. However, for this spin to be operational as a quantum bit, full quantum control is essential. Here we report the measurement of optically detected magnetic resonance and the demonstration of coherent control of a single silicon-vacancy centre spin with a microwave field. Using Ramsey interferometry, we directly measure a spin coherence time, T<sub>2</sub>*, of 115±9 ns at 3.6 K. The temperature dependence of coherence times indicates that dephasing and decay of the spin arise from single-phonon-mediated excitation between orbital branches of the ground state. Our results enable the silicon-vacancy centre spin to become a controllable resource to establish spin-photon quantum interfaces.