Anomalous spin correlations and excitonic instability of interacting 2D Weyl fermions.

Hirata, Michihiro; Ishikawa, Kyohei; Matsuno, Genki; Kobayashi, Akito; Miyagawa, Kazuya; Tamura, Masafumi; Berthier, Claude; Kanoda, Kazushi · Science · 2017

basic_science · Level V

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Abstract

The Coulomb interaction in systems of quasi-relativistic massless electrons has an unscreened long-range component at variance with conventional correlated metals. We used nuclear magnetic resonance (NMR) measurements to reveal unusual spin correlations of two-dimensional Weyl fermions in an organic material, causing a divergent increase of the Korringa ratio by a factor of 1000 upon cooling, in marked contrast to conventional metallic behavior. Combined with model calculations, we show that this divergence stems from an interaction-driven velocity renormalization that almost exclusively suppresses zero-momentum spin fluctuations. At low temperatures, the NMR relaxation rate shows an unexpected increase; numerical analyses show that this increase corresponds to internode excitonic fluctuations, a precursor to a transition from massless to massive quasiparticles.