Multidimensional photon correlation spectroscopy of cavity polaritons.
basic_science · Level V
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- Record sourced from PubMed, PMID 29386388.
- Also identified by DOI 10.1073/pnas.1719443115 and PMC identifier 5816200.
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Abstract
The strong coupling of atoms and molecules to radiation field modes in optical cavities creates dressed matter/field states known as polaritons with controllable dynamical and energy transfer properties. We propose a multidimensional optical spectroscopy technique for monitoring polariton dynamics. The response of a two-level atom to the time-dependent coupling to a single-cavity mode is monitored through time-and-frequency-resolved single-photon coincidence measurements of spontaneous emission. Polariton population and coherence dynamics and its variation with cavity photon number and controlled by gating parameters are predicted by solving the Jaynes-Cummings model.