Using controlled disorder to probe the interplay between charge order and superconductivity in NbSe<sub>2</sub>.

Cho, Kyuil; Kończykowski, M; Teknowijoyo, S; Tanatar, M A; Guss, J; Gartin, P B; Wilde, J M; Kreyssig, A et al. · Nat Commun · 2018

basic_science · Level V

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Abstract

The interplay between superconductivity and charge-density wave (CDW) in 2H-NbSe<sub>2</sub> is not fully understood despite decades of study. Artificially introduced disorder can tip the delicate balance between two competing long-range orders, and reveal the underlying interactions that give rise to them. Here we introduce disorder by electron irradiation and measure in-plane resistivity, Hall resistivity, X-ray scattering, and London penetration depth. With increasing disorder, the superconducting transition temperature, T<sub>c</sub>, varies non-monotonically, whereas the CDW transition temperature, T<sub>CDW</sub>, monotonically decreases and becomes unresolvable above a critical irradiation dose where T<sub>c</sub> drops sharply. Our results imply that the CDW order initially competes with superconductivity, but eventually assists it. We argue that at the transition where the long-range CDW order disappears, the cooperation with superconductivity is dramatically suppressed. X-ray scattering and Hall resistivity measurements reveal that the short-range CDW survives above the transition. Superconductivity persists to much higher dose levels, consistent with fully gapped superconductivity and moderate interband pairing.