High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response.

Thirimanne, H M; Jayawardena, K D G I; Parnell, A J; Bandara, R M I; Karalasingam, A; Pani, S; Huerdler, J E; Lidzey, D G et al. · Nat Commun · 2018

basic_science · Level V

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Abstract

X-ray detectors are critical to healthcare diagnostics, cancer therapy and homeland security, with many potential uses limited by system cost and/or detector dimensions. Current X-ray detector sensitivities are limited by the bulk X-ray attenuation of the materials and consequently necessitate thick crystals (~1 mm-1 cm), resulting in rigid structures, high operational voltages and high cost. Here we present a disruptive, flexible, low cost, broadband, and high sensitivity direct X-ray transduction technology produced by embedding high atomic number bismuth oxide nanoparticles in an organic bulk heterojunction. These hybrid detectors demonstrate sensitivities of 1712 µC mGy<sup>-1</sup> cm<sup>-3</sup> for "soft" X-rays and ~30 and 58 µC mGy<sup>-1</sup> cm<sup>-3</sup> under 6 and 15 MV "hard" X-rays generated from a medical linear accelerator; strongly competing with the current solid state detectors, all achieved at low bias voltages (-10 V) and low power, enabling detector operation powered by coin cell batteries.