Degassing-induced fractionation of multiple sulphur isotopes unveils post-Archaean recycled oceanic crust signal in hotspot lava.

Beaudry, Patrick; Longpré, Marc-Antoine; Economos, Rita; Wing, Boswell A; Bui, Thi Hao; Stix, John · Nat Commun · 2018

basic_science · Level V

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Abstract

Mantle source regions feeding hotspot volcanoes likely contain recycled subducted material. Anomalous sulphur (S) isotope signatures in hotspot lavas have tied ancient surface S to this deep geological cycle, but their potential modification by shallow magmatic processes has generally been overlooked. Here we present S isotope measurements in magmatic sulphides, silicate melt inclusions and matrix glasses from the recent eruption of a hotspot volcano at El Hierro, Canary Islands, which show that degassing induces strongly negative δ<sup>34</sup>S fractionation in both silicate and sulphide melts. Our results reflect the complex interplay among redox conditions, S speciation and degassing. The isotopic fractionation is mass dependent (Δ<sup>33</sup>S = 0‰), thus lacking evidence for the recycled Archaean crust signal recently identified at other hotspot volcanoes. However, the source has an enriched signature (δ<sup>34</sup>S ~ + 3‰), which supports the presence of younger <sup>34</sup>S-rich recycled oceanic material in the Canary Island mantle plume.