Paraffin-enabled graphene transfer.

Leong, Wei Sun; Wang, Haozhe; Yeo, Jingjie; Martin-Martinez, Francisco J; Zubair, Ahmad; Shen, Pin-Chun; Mao, Yunwei; Palacios, Tomas et al. · Nat Commun · 2019

basic_science · Level V

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Abstract

The performance and reliability of large-area graphene grown by chemical vapor deposition are often limited by the presence of wrinkles and the transfer-process-induced polymer residue. Here, we report a transfer approach using paraffin as a support layer, whose thermal properties, low chemical reactivity and non-covalent affinity to graphene enable transfer of wrinkle-reduced and clean large-area graphene. The paraffin-transferred graphene has smooth morphology and high electrical reliability with uniform sheet resistance with ~1% deviation over a centimeter-scale area. Electronic devices fabricated on such smooth graphene exhibit electrical performance approaching that of intrinsic graphene with small Dirac points and high carrier mobility (hole mobility = 14,215 cm<sup>2</sup> V<sup>-1</sup> s<sup>-1</sup>; electron mobility = 7438 cm<sup>2</sup> V<sup>-1</sup> s<sup>-1</sup>), without the need of further annealing treatment. The paraffin-enabled transfer process could open realms for the development of high-performance ubiquitous electronics based on large-area two-dimensional materials.