Mid infrared gas spectroscopy using efficient fiber laser driven photonic chip-based supercontinuum.

Grassani, Davide; Tagkoudi, Eirini; Guo, Hairun; Herkommer, Clemens; Yang, Fan; Kippenberg, Tobias J; Brès, Camille-Sophie · Nat Commun · 2019

basic_science · Level V

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Abstract

Directly accessing the middle infrared, the molecular functional group spectral region, via supercontinuum generation processes based on turn-key fiber lasers offers the undeniable advantage of simplicity and robustness. Recently, the assessment of the coherence of the mid-IR dispersive wave in silicon nitride (Si<sub>3</sub>N<sub>4</sub>) waveguides, pumped at telecom wavelength, established an important first step towards mid-IR frequency comb generation based on such compact systems. Yet, the spectral reach and efficiency still fall short for practical implementation. Here, we experimentally demonstrate that large cross-section Si<sub>3</sub>N<sub>4</sub> waveguides pumped with 2 μm fs-fiber laser can reach the important spectroscopic spectral region in the 3-4 μm range, with up to 35% power conversion and milliwatt-level output powers. As a proof of principle, we use this source for detection of C<sub>2</sub>H<sub>2</sub> by absorption spectroscopy. Such result makes these sources suitable candidate for compact, chip-integrated spectroscopic and sensing applications.