Efficient Coupling of an Ensemble of Nitrogen Vacancy Center to the Mode of a High-Q, Si<sub>3</sub>N<sub>4</sub> Photonic Crystal Cavity.

Fehler, Konstantin G; Ovvyan, Anna P; Gruhler, Nico; Pernice, Wolfram H P; Kubanek, Alexander · ACS Nano · 2019

basic_science · Level V

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Abstract

Integrated nanophotonics is an emerging field with high potential for quantum technology applications such as quantum sensing or quantum networks. A desired photonics platform is Si<sub>3</sub>N<sub>4</sub> due to low-photon loss and well-established fabrication techniques. However, quantum optics applications are not yet established. Here, we investigate an approach toward Si<sub>3</sub>N<sub>4</sub>-based quantum photonics utilizing a crossed waveguide, pump-probe design. The platform enables efficient, on-chip excitation, strong background suppression, and at the same time, efficient coupling to the mode of a high- Q photonic crystal cavity. The freestanding photonic crystal cavities reach high Q-factors up to 47 × 10<sup>3</sup>. To test our platform, we positioned an ensemble of negatively charged nitrogen vacancy centers located in a nanodiamond within the interaction zone of the photonic crystal cavity. We quantify the efficiency of the coupling with the β<sub>λ</sub>-factor reaching values as large as 0.71. We further demonstrate on-chip excitation of the quantum emitter with strong suppression (∼20 dB) of the background fluorescence. Our results unfold the potential to utilize negatively charged nitrogen vacancy centers in nanodiamonds and Si<sub>3</sub>N<sub>4</sub> platforms as an efficient, on-chip spin-photon interface in quantum photonics experiments.