2D semiconductor nonlinear plasmonic modulators.

Klein, Matthew; Badada, Bekele H; Binder, Rolf; Alfrey, Adam; McKie, Max; Koehler, Michael R; Mandrus, David G; Taniguchi, Takashi et al. · Nat Commun · 2019

basic_science · Level V

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Abstract

A plasmonic modulator is a device that controls the amplitude or phase of propagating plasmons. In a pure plasmonic modulator, the presence or absence of a plasmonic pump wave controls the amplitude of a plasmonic probe wave through a channel. This control has to be mediated by an interaction between disparate plasmonic waves, typically requiring the integration of a nonlinear material. In this work, we demonstrate a 2D semiconductor nonlinear plasmonic modulator based on a WSe<sub>2</sub> monolayer integrated on top of a lithographically defined metallic waveguide. We utilize the strong interaction between the surface plasmon polaritons (SPPs) and excitons in the WSe<sub>2</sub> to give a 73 % change in transmission through the device. We demonstrate control of the propagating SPPs using both optical and SPP pumps, realizing a 2D semiconductor nonlinear plasmonic modulator, with an ultrafast response time of 290 fs.