Nanoscale mapping of quasiparticle band alignment.
basic_science · Level V
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- Record sourced from PubMed, PMID 31337765.
- Also identified by DOI 10.1038/s41467-019-11253-2 and PMC identifier 6650412.
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Abstract
Control of atomic-scale interfaces between materials with distinct electronic structures is crucial for the design and fabrication of most electronic devices. In the case of two-dimensional materials, disparate electronic structures can be realized even within a single uniform sheet, merely by locally applying different vertical gate voltages. Here, we utilize the inherently nano-structured single layer and bilayer graphene on silicon carbide to investigate lateral electronic structure variations in an adjacent single layer of tungsten disulfide (WS<sub>2</sub>). The electronic band alignments are mapped in energy and momentum space using angle-resolved photoemission with a spatial resolution on the order of 500 nm (nanoARPES). We find that the WS<sub>2</sub> band offsets track the work function of the underlying single layer and bilayer graphene, and we relate such changes to observed lateral patterns of exciton and trion luminescence from WS<sub>2</sub>.