Cavity-control of interlayer excitons in van der Waals heterostructures.

Förg, Michael; Colombier, Léo; Patel, Robin K; Lindlau, Jessica; Mohite, Aditya D; Yamaguchi, Hisato; Glazov, Mikhail M; Hunger, David et al. · Nat Commun · 2019

basic_science · Level V

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Abstract

Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing spatially indirect excitons with a permanent electric dipole moment in heterobilayer crystals promise realizations of exciton-polariton gases and condensates with inherent dipolar interactions. Here, we implement cavity-control of interlayer excitons in vertical MoSe<sub>2</sub>-WSe<sub>2</sub> heterostructures. Our experiments demonstrate the Purcell effect for heterobilayer emission in cavity-modified photonic environments, and quantify the light-matter coupling strength of interlayer excitons. The results will facilitate further developments of dipolar exciton-polariton gases and condensates in hybrid cavity - van der Waals heterostructure systems.