Attosecond optoelectronic field measurement in solids.

Sederberg, Shawn; Zimin, Dmitry; Keiber, Sabine; Siegrist, Florian; Wismer, Michael S; Yakovlev, Vladislav S; Floss, Isabella; Lemell, Christoph et al. · Nat Commun · 2020

basic_science · Level V

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Abstract

The sub-cycle interaction of light and matter is one of the key frontiers of inquiry made accessible by attosecond science. Here, we show that when light excites a pair of charge carriers inside of a solid, the transition probability is strongly localized to instants slightly after the extrema of the electric field. The extreme temporal localization is utilized in a simple electronic circuit to record the waveforms of infrared to ultraviolet light fields. This form of petahertz-bandwidth field metrology gives access to both the modulated transition probability and its temporal offset from the laser field, providing sub-fs temporal precision in reconstructing the sub-cycle electronic response of a solid state structure.