Ambient weathering of magnesium oxide for CO<sub>2</sub> removal from air.

McQueen, Noah; Kelemen, Peter; Dipple, Greg; Renforth, Phil; Wilcox, Jennifer · Nat Commun · 2020

basic_science · Level V

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Abstract

To avoid dangerous climate change, new technologies must remove billions of tonnes of CO<sub>2</sub> from the atmosphere every year by mid-century. Here we detail a land-based enhanced weathering cycle utilizing magnesite (MgCO<sub>3</sub>) feedstock to repeatedly capture CO<sub>2</sub> from the atmosphere. In this process, MgCO<sub>3</sub> is calcined, producing caustic magnesia (MgO) and high-purity CO<sub>2</sub>. This MgO is spread over land to carbonate for a year by reacting with atmospheric CO<sub>2</sub>. The carbonate minerals are then recollected and re-calcined. The reproduced MgO is spread over land to carbonate again. We show this process could cost approximately $46-159 tCO<sub>2</sub><sup>-1</sup> net removed from the atmosphere, considering grid and solar electricity without post-processing costs. This technology may achieve lower costs than projections for more extensively engineered Direct Air Capture methods. It has the scalable potential to remove at least 2-3 GtCO<sub>2</sub> year<sup>-1</sup>, and may make a meaningful contribution to mitigating climate change.