A two-lane mechanism for selective biological ammonium transport.

Williamson, Gordon; Tamburrino, Giulia; Bizior, Adriana; Boeckstaens, Mélanie; Dias Mirandela, Gaëtan; Bage, Marcus G; Pisliakov, Andrei; Ives, Callum M et al. · Elife · 2020

basic_science · Level V

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Abstract

The transport of charged molecules across biological membranes faces the dual problem of accommodating charges in a highly hydrophobic environment while maintaining selective substrate translocation. This has been the subject of a particular controversy for the exchange of ammonium across cellular membranes, an essential process in all domains of life. Ammonium transport is mediated by the ubiquitous Amt/Mep/Rh transporters that includes the human Rhesus factors. Here, using a combination of electrophysiology, yeast functional complementation and extended molecular dynamics simulations, we reveal a unique two-lane pathway for electrogenic NH<sub>4</sub><sup>+</sup> transport in two archetypal members of the family, the transporters AmtB from <i>Escherichia coli</i> and Rh50 from <i>Nitrosomonas europaea</i>. The pathway underpins a mechanism by which charged H<sup>+</sup> and neutral NH<sub>3</sub> are carried separately across the membrane after NH<sub>4</sub><sup>+</sup> deprotonation. This mechanism defines a new principle of achieving transport selectivity against competing ions in a biological transport process.

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