Microchannels with Self-Pumping Walls.

Yu, Tingting; Athanassiadis, Athanasios G; Popescu, Mihail N; Chikkadi, Vijayakumar; Güth, Achim; Singh, Dhruv P; Qiu, Tian; Fischer, Peer · ACS Nano · 2020

basic_science · Level V

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Abstract

When asymmetric Janus micromotors are immobilized on a surface, they act as chemically powered micropumps, turning chemical energy from the fluid into a bulk flow. However, such pumps have previously produced only localized recirculating flows, which cannot be used to pump fluid in one direction. Here, we demonstrate that an array of three-dimensional, photochemically active Au/TiO<sub>2</sub> Janus pillars can pump water. Upon UV illumination, a water-splitting reaction rapidly creates a directional bulk flow above the active surface. By lining a 2D microchannel with such active surfaces, various flow profiles are created within the channels. Analytical and numerical models of a channel with active surfaces predict flow profiles that agree very well with the experimental results. The light-driven active surfaces provide a way to wirelessly pump fluids at small scales and could be used for real-time, localized flow control in complex microfluidic networks.