Fabrication of a novel magnetic topological heterostructure and temperature evolution of its massive Dirac cone.

Hirahara, T; Otrokov, M M; Sasaki, T T; Sumida, K; Tomohiro, Y; Kusaka, S; Okuyama, Y; Ichinokura, S et al. · Nat Commun · 2020

basic_science · Level V

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Abstract

Materials that possess nontrivial topology and magnetism is known to exhibit exotic quantum phenomena such as the quantum anomalous Hall effect. Here, we fabricate a novel magnetic topological heterostructure Mn<sub>4</sub>Bi<sub>2</sub>Te<sub>7</sub>/Bi<sub>2</sub>Te<sub>3</sub> where multiple magnetic layers are inserted into the topmost quintuple layer of the original topological insulator Bi<sub>2</sub>Te<sub>3</sub>. A massive Dirac cone (DC) with a gap of 40-75 meV at 16 K is observed. By tracing the temperature evolution, this gap is shown to gradually decrease with increasing temperature and a blunt transition from a massive to a massless DC occurs around 200-250 K. Structural analysis shows that the samples also contain MnBi<sub>2</sub>Te<sub>4</sub>/Bi<sub>2</sub>Te<sub>3</sub>. Magnetic measurements show that there are two distinct Mn components in the system that corresponds to the two heterostructures; MnBi<sub>2</sub>Te<sub>4</sub>/Bi<sub>2</sub>Te<sub>3</sub> is paramagnetic at 6 K while Mn<sub>4</sub>Bi<sub>2</sub>Te<sub>7</sub>/Bi<sub>2</sub>Te<sub>3</sub> is ferromagnetic with a negative hysteresis (critical temperature  ~20 K). This novel heterostructure is potentially important for future device applications.