Thermal Hall conductivity in the cuprate Mott insulators Nd<sub>2</sub>CuO<sub>4</sub> and Sr<sub>2</sub>CuO<sub>2</sub>Cl<sub>2</sub>.

Boulanger, Marie-Eve; Grissonnanche, Gaël; Badoux, Sven; Allaire, Andréanne; Lefrançois, Étienne; Legros, Anaëlle; Gourgout, Adrien; Dion, Maxime et al. · Nat Commun · 2020

basic_science · Level V

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Abstract

The heat carriers responsible for the unexpectedly large thermal Hall conductivity of the cuprate Mott insulator La<sub>2</sub>CuO<sub>4</sub> were recently shown to be phonons. However, the mechanism by which phonons in cuprates acquire chirality in a magnetic field is still unknown. Here, we report a similar thermal Hall conductivity in two cuprate Mott insulators with significantly different crystal structures and magnetic orders - Nd<sub>2</sub>CuO<sub>4</sub> and Sr<sub>2</sub>CuO<sub>2</sub>Cl<sub>2</sub> - and show that two potential mechanisms can be excluded - the scattering of phonons by rare-earth impurities and by structural domains. Our comparative study further reveals that orthorhombicity, apical oxygens, the tilting of oxygen octahedra and the canting of spins out of the CuO<sub>2</sub> planes are not essential to the mechanism of chirality. Our findings point to a chiral mechanism coming from a coupling of acoustic phonons to the intrinsic excitations of the CuO<sub>2</sub> planes.