Lithography-free IR polarization converters via orthogonal in-plane phonons in α-MoO<sub>3</sub> flakes.

Abedini Dereshgi, Sina; Folland, Thomas G; Murthy, Akshay A; Song, Xianglian; Tanriover, Ibrahim; Dravid, Vinayak P; Caldwell, Joshua D; Aydin, Koray · Nat Commun · 2020

basic_science · Level V

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Abstract

Exploiting polaritons in natural vdW materials has been successful in achieving extreme light confinement and low-loss optical devices and enabling simplified device integration. Recently, α-MoO<sub>3</sub> has been reported as a semiconducting biaxial vdW material capable of sustaining naturally orthogonal in-plane phonon polariton modes in IR. In this study, we investigate the polarization-dependent optical characteristics of cavities formed using α-MoO<sub>3</sub> to extend the degrees of freedom in the design of IR photonic components exploiting the in-plane anisotropy of this material. Polarization-dependent absorption over 80% in a multilayer Fabry-Perot structure with α-MoO<sub>3</sub> is reported without the need for nanoscale fabrication on the α-MoO<sub>3</sub>. We observe coupling between the α-MoO<sub>3</sub> optical phonons and the Fabry-Perot cavity resonances. Using cross-polarized reflectance spectroscopy we show that the strong birefringence results in 15% of the total power converted into the orthogonal polarization with respect to incident wave. These findings can open new avenues in the quest for polarization filters and low-loss, integrated planar IR photonics and in dictating polarization control.