High-Quality All-Inorganic Perovskite CsPbBr<sub>3</sub> Microsheet Crystals as Low-Loss Subwavelength Exciton-Polariton Waveguides.
basic_science · Level V
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- Record sourced from PubMed, PMID 33560855.
- Also identified by DOI 10.1021/acs.nanolett.0c04908.
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Abstract
Nanostructured all-inorganic metal halide perovskites have attracted considerable attention due to their outstanding photonic and optoelectronic properties. Particularly, they can exhibit room-temperature exciton-polaritons (EPs) capable of confining electromagnetic fields down to the subwavelength scale, enabling efficient light harvesting and guiding. However, a real-space nanoimaging study of the EPs in perovskite crystals is still absent. Additionally, few studies focused on the ambient-pressure and reliable fabrication of large-area CsPbBr<sub>3</sub> microsheets. Here, CsPbBr<sub>3</sub> orthorhombic microsheet single crystals were successfully synthesized under ambient pressure. Their EPs were examined using a real-space nanoimaging technique, which reveal EP waveguide modes spanning the visible to near-infrared spectral region. The EPs exhibit a sufficient long propagation length of over 16 μm and a very low propagation loss of less than 0.072 dB·μm<sup>-1</sup>. These results demonstrate the potential applications of CsPbBr<sub>3</sub> microsheets as subwavelength waveguides in integrated optics.