Plasmonic Split-Trench Resonator for Trapping and Sensing.

Yoo, Daehan; Barik, Avijit; de León-Pérez, Fernando; Mohr, Daniel A; Pelton, Matthew; Martín-Moreno, Luis; Oh, Sang-Hyun · ACS Nano · 2021

basic_science · Level V

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Abstract

On-chip integration of plasmonics and electronics can benefit a broad range of applications in biosensing, signal processing, and optoelectronics. A key requirement is a chip-scale manufacturing method. Here, we demonstrate a split-trench resonator platform that combines a high-quality-factor resonant plasmonic biosensor with radio frequency (RF) nanogap tweezers. The split-trench resonator can simultaneously serve as a dielectrophoretic trap and a nanoplasmonic sensor. Trapping is accomplished by applying an RF electrical bias across a 10 nm gap, thereby either attracting or repelling analytes. Trapped analytes are detected in a label-free manner using refractive-index sensing, enabled by interference between surface-plasmon standing waves in the trench and light transmitted through the gap. This active sample concentration mechanism enables detection of nanoparticles and proteins at a concentration as low as 10 pM. We can manufacture centimeter-long split-trench cavity resonators with high throughput <i>via</i> photolithography and atomic layer deposition, toward practical applications in biosensing, spectroscopy, and optoelectronics.