Purcell-like Enhancement of Electron-Phonon Interactions in Long-Period Superlattices: Linear-Temperature Resistivity and Cooling Power.
basic_science · Level V
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- Record sourced from PubMed, PMID 34515488.
- Also identified by DOI 10.1021/acs.nanolett.1c00565.
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Abstract
In the Purcell effect, the efficiency of optical emitters is enhanced by reducing the optical mode volume. Here we predict an analogous enhancement for electron-phonon (el-ph) scattering, achieved by compressing the electronic Wannier orbitals. Reshaped Wannier orbitals are a prominent attribute of graphene moiré superlattices, where the orbital size is tunable by the twist angle. A reduction in the orbital size leads to an enhancement in the el-ph interaction strength, yielding the values considerably larger than those in pristine monolayer graphene. The enhanced coupling boosts the el-ph scattering rates, pushing them above the values expected for the flat-band-enhanced density of electronic states. The enhanced phonon emission and scattering rates are manifested through the observables such as the electron-lattice cooling and the linear-temperature (<i>T</i>) resistivity, both of which are directly tunable by the moiré twist angle.