Autumn destabilization of deep porewater CO<sub>2</sub> store in a northern peatland driven by turbulent diffusion.

Campeau, A; Vachon, D; Bishop, K; Nilsson, M B; Wallin, M B · Nat Commun · 2021

basic_science · Level V

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Abstract

The deep porewater of northern peatlands stores large amounts of carbon dioxide (CO<sub>2</sub>). This store is viewed as a stable feature in the peatland CO<sub>2</sub> cycle. Here, we report large and rapid fluctuations in deep porewater CO<sub>2</sub> concentration recurring every autumn over four consecutive years in a boreal peatland. Estimates of the vertical diffusion of heat indicate that CO<sub>2</sub> diffusion occurs at the turbulent rather than molecular rate. The weakening of porewater thermal stratification in autumn likely increases turbulent diffusion, thus fostering a rapid diffusion of deeper porewater CO<sub>2</sub> towards the surface where net losses occur. This phenomenon periodically decreases the peat porewater CO<sub>2</sub> store by between 29 and 90 g C m<sup>-2</sup> throughout autumn, which is comparable to the peatland's annual C-sink. Our results establish the need to consider the role of turbulent diffusion in regularly destabilizing the CO<sub>2</sub> store in peat porewater.